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Together, these elements indicate a very strong patterning in the S-HC8 system, reaching almost a perfectly stabilized and strongly oriented water wire. The chiral compatibility of the S-HC8 system with the L-type lipids probably better stabilizes the respective I-quartet channel that adopts a conformation, where water molecules are more strongly associated than in bulk water. The R-HC8 system maintains a strong dipolar orientation with fine-tuned interactions along the water wire, comparable energetics with respect to bulk water, and hence an increased mobility along a structured water path. The HC8 channels are slightly destabilized compared with bulk water and do not form stable wire arrangements in the unsupported lipid bilayers.

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DFT calculation was performed by using the CP2K package. The Perdew-Burke-Ernzerhof functional with Grimme D3 correction was used to describe the system. Unrestricted Kohn-Sham DFT was used as the electronic structure method in the framework of the Gaussian and plane-wave method. The Goedecker-Teter-Hutter (GTH) pseudopotentials and DZVP-MOLOPT-GTH basis sets were used to describe the molecules. A plane-wave energy cutoff of 500 rydbergs was used.

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OSL and IRSL dates indicate minima ages of deglaciation and pro-glacial lake drainage (55), and calibrated 14C dates indicate minima dates for fauna and vegetation (12, 35, 61, 63, 80–82). Demic expansion estimates of Native American ancestors from (13). All dates are shown with 1 SD.

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