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[H01L] SEMICONDUCTOR DEVICES; ELECTRIC SOLID STATE DEVICES NOT OTHERWISE PROVIDED FOR (use of semiconductor devices for measuring G01; resistors in general H01C; magnets, inductors, transformers H01F; capacitors in general H01G; electrolytic devices H01G 9/00; batteries, accumulators H01M; waveguides, resonators, or lines of the waveguide type H01P; line connectors, current collectors H01R; stimulated-emission devices H01S; electromechanical resonators H03H; loudspeakers, microphones, gramophone pick-ups or like acoustic electromechanical transducers H04R; electric light sources in general H05B; printed circuits, hybrid circuits, casings or constructional details of electrical apparatus, manufacture of assemblages of electrical components H05K; use of semiconductor devices in circuits having a particular application, see the subclass for the application) [2]

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Inventor(s): John B. Adrain (Frisco, TX) Assignee(s): UNASSIGNED Law Firm: Bodi Law LLC (no location found) Application No., Date, Speed: 15050639 on 02/23/2016 (1022 days app to issue)

Remarkably, the intensity of the Raman peak at 1530 cm−1, corresponding to the in-plane ring symmetric nonmetal bound N–C stretch of CuPc, was used as a reference peak for further research (table S1) (30). It was found that MGT had better enhancement for CuPc compared with MG, an effect that could be ascribed mainly to the addition of a semiconductor, TiO2, to the GO-containing platform. The EF value of MGT for CuPc molecules was calculated to be as high as 8.08 × 106 (for calculation details, see Materials and Methods), which was much higher than that of graphene alone (47.3) (29) and the highest EF value (6.62 × 105) of plasmon-free materials reported to date (31). Given that the wavelength of the excitation laser used for Raman measurement in this work was 633 nm, which is close to the ultraviolet-visible (UV-vis) absorption peak of CuPc (fig. S4D), the high EF value may be attributed to the SERS effect of CuPc (32). After the excitation laser wavelength was adjusted to either 532 or 780 nm, we observed relatively weak absorption for CuPc molecules. Compared with absorption under 633-nm excitation, an obvious decline (~44%) in the Raman intensity of CuPc was observed under 532-nm irradiation, while no obvious Raman signals were obtained under 780 nm (fig. S4E). The results indicate that resonance Raman effect plays an important role in Raman enhancement.

A barrier to develop bioinspired synthetic systems lies in deciphering the complexity of natural systems. The findings presented here increase our understanding toward biomimicking the water structure within the extremely efficient AQPs, which remains an important exploratory challenge. The I-quartet artificial water channel provides remarkable combinations of functions very close to those encountered in natural AQPs and provides a simplified system, where the structural alignment of confined water can be elucidated and quantified. Our comprehensive study shows that self-assembled I-quartets embedded into lipid bilayers form highly ordered structures containing chiral dipolar oriented water wires. Our complementary x-ray single-crystal, QCM-D, MD, and nonlinear SFG spectroscopic studies presented here provide the first insight into the hydrogen-bonded structure and dipolar orientation of the water molecules inside the I-quartet channels in the lipid membrane environment at a molecular level.

[B29C] SHAPING OR JOINING OF PLASTICS; SHAPING OF MATERIAL IN A PLASTIC STATE, NOT OTHERWISE PROVIDED FOR; AFTER-TREATMENT OF THE SHAPED PRODUCTS, e.g. REPAIRING (making preforms B29B 11/00; making laminated products by combining previously unconnected layers which become one product whose layers will remain together B32B 37/00-B32B 41/00) [4]

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